A033-0005
Southern Ocean latitudinal gradients of Cloud Condensation Nuclei
Abstract:
Aerosol data (CN10 and CCN at numerous supersaturations) free from platform exhaust, were divided into 5o latitudinal bins. The northern-most bin (40-45oS) was found, unsurprisingly, to exhibit the highest concentrations (CCN0.2 ~100 cm-3; CCN0.5 ~250 cm-3; CN10 ~600 cm-3), with back-trajectory analyses revealing substantial influence from continental sources of Tasmania and to a lesser extent, Victoria. Latitudinal bins between 45-65oS were reasonably consistent (CCN0.2 ~ 100 cm-3; CCN0.5 150 cm-3; CN10 ~300 cm-3), with trajectories showing a marine boundary layer source region from the south-west. CCN measurements in this latitudinal range agreed with concurrent measurements at Macquarie Island and at Cape Grim. The southern-most latitudinal bin (65-70oS) showed a distinct change in populations, with increases in aerosol concentrations (CCN0.2 ~130 cm-3; CCN0.5 250 cm-3; CN10 ~350 cm-3) and CCN/CN10 ratios, consistent with previous measurements resulting from transitioning across the atmospheric polar front. Analyses to further understand these changes showed corresponding increases in sulfate aerosols, decreases in sea-salt aerosol and decreases in both wind speed and precipitation influence.
This dataset is important observational data that will help verify climate and earth system models, and constrain satellite data. These data also help to untangle the mystery of the compositional changes consistently observed across the atmospheric polar front.